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          天然產物合成化學

            天然產物是自然界長期進化的物質實體,是生物活性物質和實用藥物發現的重要源泉。然而,這些天然產物并不是取之不盡、用之不竭,那些具有很好生理活性的天然產物往往在其載體如植物、動物、微生物中的含量稀少。正是由于這些活性天然產物的自然來源十分有限,人類對其藥用天然資源的過度采伐,加上自然環境的退化等原因,導致相關特種生物資源的逐漸瀕危,從而使生物資源的可持續利用及環境可持續發展正在面臨一系列的難題。

            為了天然藥用資源的可持續利用以及環境、生態保護,從易得的原料出發,開展活性“天然產物化學合成研究”是一條有效的科學途徑。對于尋找特有生物資源的替代物質、減少珍稀藥用資源的毀滅性采伐,尤其是珍稀特種生物資源的保護,具有長遠的戰略意義。

            天然產物化學合成是有機化學研究中最活躍、最具挑戰性的研究領域,它在很大程度上反映了一個國家有機化學研究的水平和實力。重要有機化合物的合成化學不僅為各種功能分子的人工合成提供了高效、經濟的工藝和技術,同時極大地推動了有機化學理論和方法的發展。歷史上許多重要的有機化學理論、化學反應和試劑都是從復雜有機化合物的全合成研究中誕生和發展的。

            本次創新團隊將主要以生物活性天然產物為研究對象,針對它們的化學全合成以及相關合成方法問題,從策略設計的角度出發,發展一些導向天然產物合成的方法學,并重點進行一系列天然產物化學合成研究,在更高層次上凸顯“天然產物合成”對有機化學學科發展的帶動、引領。

            團隊的主要研究方向包括以下兩個方面:
            (1)天然產物化學合成研究;
            (2)導向天然產物合成的有機合成方法學研究。

            該團隊入選以來所取得的主要成績:
            “天然產物合成化學”長江學者創新團隊依托蘭州大學功能有機分子化學國家重點實驗室和有機化學國家重點學科,結合重點實驗室優勢研究發展方向,在“天然產物合成化學”方面形成了自身的研究特色。以一系列具有重要生物活性的天然產物為研究對象,圍繞“天然產物合成化學”這一主題,重點開展“天然產物全合成研究”與“導向天然產物合成的有機合成方法學研究”。團隊獲資助一年以來,在有機合成領域取得了一系列階段性的研究成果,對三萜Simaroubin、虎皮楠生物堿、石松生物堿Fawcettimine、萜類生物堿Sculponeatin N、、Actinophyllic acid等天然產物的合成研究均取得了一定的結果,方法學領域開展了有機化學中碳-碳、碳-雜鍵構筑轉化的研究。項目執行第一年已發表多篇高水平研究論文,并且該年度樊春安教授獲得2012年“Thieme Chemistry Journals Award”,翟宏斌教授獲得2012年“Asian Core Program Lectureship Award”。

          團隊負責人簡介

            翟宏斌,男,漢族,1966年10月出生,江蘇揚中人,現任蘭州大學功能有機分子化學國家重點實驗室主任,博士,二級教授,2006年獲得國家杰出青年科學基金,2009年入選 “百千萬人才工程”國家級人選。1981.9–1985.6:北京大學技術物理系應用化學專業,學士學位。1989.10–1995.6:美國俄亥俄州立大學化學系有機化學專業,博士學位。 1996.2–1997.3:美國俄亥俄州立大學藥學院藥物化學專業,博士后,導師:Albert H. Soloway。 1998.4–2000.3:美國加里福尼亞大學伯克利分校化學系,博士后,導師:Henry Rapoport。 2000.5–2010.3:中科院上海有機所研究員,博士生導師。曾任中科院上海有機所現代有機合成化學研究室室主任。 2004.5–2006.2:(兼任)國家自然科學基金委化學科學部化學生物學流動項目主任。 2010.4–目前:蘭州大學萃英特聘教授,博士生導師。現任蘭州大學功能有機分子化學國家重點實驗室主任、兼任“蘭州大學學報(自然科學版)”副主編。

             翟宏斌教授主要學術成就和獲獎情況:在苦艾素首次仿生不對稱全合成(J. Am. Chem. Soc. 2005)實現之后,翟宏斌教授及其團隊圍繞天然產物全合成領域中若干國際熱門研究課題,近期完成了Merrilactone A、(-)-Jiadifenin 和(-)-Nakadomarin A 等一系列重要天然產物的簡潔高效全合成。所涉及天然產物分子通常兼具復雜環系結構和重要生物活性,合成工作可望為創新藥物研發提供藥物先導化合物。近期代表性工作:具有復雜籠狀結構和神經營養活性的倍半萜Merrilactone A (Angew. Chem., Int. Ed. 2012)和(-)-Jiadifenin(Angew. Chem., Int. Ed. 2012)的全合成,發表后分別被Chin. J. Org. Chem.和Synfacts 作為亮點介紹,并受邀將為Synthesis 撰寫Feature Article。迄今發表論文50 余篇;申請中國專利2項均獲授權。

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